[gpaw-users] problem of electronic convergence

Vladislav Ivanistsev olunet at gmail.com
Thu Jan 17 15:57:42 CET 2013


yes, here is the output


On Thu, Jan 17, 2013 at 2:35 PM, Ask Hjorth Larsen <asklarsen at gmail.com>wrote:

> Dear Vladislav
>
> Can you send a text output file showing it not converging?
>
> Regards
> Ask
>
> 2013/1/17 Vladislav Ivanistsev <olunet at gmail.com>:
> > Dear Ask,
> > a while ago you have "magically" resolved a problem of electronic
> > convergence in BN or Graphene slab. I'm also having a problem with
> > convergence for several systems. One is attached. Could you please take a
> > look and provide some explanation on how to converge similar
> calculations.
> > I'm using GPAW 0.9
> >
> > Many thanks,
> > Vladislav
>
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cores: 24

Memory estimate
---------------
Process memory now: 52.03 MiB
Calculator  627.55 MiB
    Density  35.20 MiB
        Arrays  18.35 MiB
        Localized functions  10.01 MiB
        Mixer  6.84 MiB
    Hamiltonian  26.47 MiB
        Arrays  12.01 MiB
        XC  0.00 MiB
        Poisson  13.71 MiB
        vbar  0.75 MiB
    Wavefunctions  565.88 MiB
        Arrays psit_nG  186.10 MiB
        Eigensolver  190.89 MiB
        Projectors  1.63 MiB
        Overlap op  187.27 MiB

Positions:
  0 Bi   11.8100   14.1741    6.5900
  1 Bi   16.3500   14.1741    6.5900
  2 Bi    7.2700   14.1741    6.5900
  3 Bi   14.0800   18.1058    6.5900
  4 Bi    9.5400   18.1058    6.5900
  5 Bi   14.0800   10.2423    6.5900
  6 Bi    9.5400   10.2423    6.5900
  7 Bi   18.6200   10.2423    6.5900
  8 Bi    5.0000   10.2423    6.5900
  9 Bi   11.8100    6.3106    6.5900
 10 Bi   16.3500    6.3106    6.5900
 11 Bi    7.2700    6.3106    6.5900
 12 Bi   11.8100    8.9317    5.0000
 13 Bi   16.3500    8.9317    5.0000
 14 Bi    7.2700    8.9317    5.0000
 15 Bi   14.0800    5.0000    5.0000
 16 Bi    9.5400    5.0000    5.0000
 17 Bi   14.0800   12.8635    5.0000
 18 Bi    9.5400   12.8635    5.0000
 19 Bi   18.6200   12.8635    5.0000
 20 Bi    5.0000   12.8635    5.0000
 21 Bi   11.8100   16.7952    5.0000
 22 Bi   16.3500   16.7952    5.0000
 23 Bi    7.2700   16.7952    5.0000
 24 B    10.8438   12.1633    9.6639
 25 F    11.5917   11.6701    8.5070
 26 F    10.5711   11.0490   10.4741
 27 F    11.6970   13.0558   10.3363
 28 F     9.6891   12.7822    9.2129
 29 C    13.8625   10.7888   10.3503
 30 N    14.9500   11.3643   10.8720
 31 N    13.7146    9.5783   10.8965
 32 C    15.5190   10.4895   11.7786
 33 C    14.7475    9.3689   11.7905
 34 H    13.2000   11.2278    9.6216
 35 C    15.4205   12.7289   10.5534
 36 C    12.6583    8.6222   10.5375
 37 H    16.4110   10.7347   12.3283
 38 H    14.8439    8.4539   12.3485
 39 C    14.7806   13.7946   11.4367
 40 H    16.5071   12.7131   10.6517
 41 H    15.1958   12.9026    9.5007
 42 H    11.7588    9.1807   10.2851
 43 H    12.4606    7.9843   11.3974
 44 H    12.9835    8.0138    9.6919
 45 H    13.6977   13.8061   11.3057
 46 H    15.1752   14.7717   11.1478
 47 H    15.0141   13.6312   12.4918

               .---------------------------------------------------------.  
              /|                                                         |  
             / |                                                         |  
            /  |                                                         |  
           /   |                                                         |  
          /    |                                                         |  
         /     |                                                         |  
        /      |                                                         |  
       /       |                                                         |  
      /        |                                                         |  
     /         |                                                         |  
    /          |                                                         |  
   /           |                              H                          |  
  /            |                           H  CH                         |  
 *             |                                H                        |  
 |             |                      F    H C C H                       |  
 |             |                 FFBH   N C   HBi                        |  
 |             |                   H C  H                                |  
 |             |                     F                                   |  
 |             |           BiBi       HBii        Bii                    |  
 |             |                                                         |  
 |             .---BiBi--------Bii--------Bii--------BiBi----------------.  
 |            /                                                         /   
 |           /         Bi         Bi         Bi                        /    
 |          /           Bi         Bi          Bi                     /     
 |         /                                                         /      
 |        /                Bi          Bi                           /       
 |       /                                                         /        
 |      /                                                         /         
 |     /                                                         /          
 |    /                                                         /           
 |   /                                                         /            
 |  /                                                         /             
 | /                                                         /              
 |/                                                         /               
 *---------------------------------------------------------*                

Unit Cell:
           Periodic     X           Y           Z      Points  Spacing
  --------------------------------------------------------------------
  1. axis:    no    23.620000    0.000000    0.000000   148     0.1596
  2. axis:    no     0.000000   23.105800    0.000000   144     0.1605
  3. axis:    no     0.000000    0.000000   17.491785   108     0.1620

Bi-setup:
  name   : Bismuth
  id     : 310b14fa21bbc5db6855c438301d06aa
  Z      : 83
  valence: 15
  core   : 68
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/Bi.RPBE.gz
  cutoffs: 1.16(comp), 2.23(filt), 2.33(core), lmax=2
  valence states:
            energy   radius
    6s(2)  -14.318   1.164
    6p(3)   -4.518   1.270
    5d(10) -27.109   1.164
    *s      12.893   1.164
    *p      22.693   1.270
    *d       0.102   1.164

Using partial waves for Bi as LCAO basis

B-setup:
  name   : Boron
  id     : 4c085ebb9e6144015c26e053032a3a9b
  Z      : 5
  valence: 3
  core   : 2
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/B.RPBE.gz
  cutoffs: 0.64(comp), 1.14(filt), 1.38(core), lmax=2
  valence states:
            energy   radius
    2s(2)   -9.489   0.635
    2p(1)   -3.587   0.635
    *s      17.723   0.635
    *p      23.625   0.635
    *d       0.000   0.635

Using partial waves for B as LCAO basis

F-setup:
  name   : Fluorine
  id     : 96d5c0c6d5d6dd1db009b0a4cc47c564
  Z      : 9
  valence: 7
  core   : 2
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/F.RPBE.gz
  cutoffs: 0.64(comp), 1.14(filt), 0.74(core), lmax=2
  valence states:
            energy   radius
    2s(2)  -29.979   0.635
    2p(5)  -11.057   0.635
    *s      -2.768   0.635
    *p      16.154   0.635
    *d       0.000   0.635

Using partial waves for F as LCAO basis

C-setup:
  name   : Carbon
  id     : 5e1162da8ccece2d28d8b78a977ec463
  Z      : 6
  valence: 4
  core   : 2
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/C.RPBE.gz
  cutoffs: 0.64(comp), 1.14(filt), 1.14(core), lmax=2
  valence states:
            energy   radius
    2s(2)  -13.815   0.635
    2p(2)   -5.254   0.635
    *s      13.396   0.635
    *p      21.957   0.635
    *d       0.000   0.635

LCAO basis set for C:
  Name: dzp
  Basis set was loaded from file /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/C.dzp.basis.gz
  Number of radial functions: 5
  Number of spherical harmonics: 13
    l=0, rc=5.5469 Bohr: 2s-sz confined orbital
    l=1, rc=6.6719 Bohr: 2p-sz confined orbital
    l=0, rc=3.0312 Bohr: 2s-dz split-valence wave
    l=1, rc=3.7500 Bohr: 2p-dz split-valence wave
    l=2, rc=6.6719 Bohr: d-type Gaussian polarization

N-setup:
  name   : Nitrogen
  id     : b7ab9cfe07f82faf48b1d9b642f2a371
  Z      : 7
  valence: 5
  core   : 2
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/N.RPBE.gz
  cutoffs: 0.58(comp), 1.03(filt), 0.96(core), lmax=2
  valence states:
            energy   radius
    2s(2)  -18.658   0.582
    2p(3)   -7.050   0.582
    *s       8.553   0.582
    *p      20.161   0.582
    *d       0.000   0.582

LCAO basis set for N:
  Name: dzp
  Basis set was loaded from file /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/N.dzp.basis.gz
  Number of radial functions: 5
  Number of spherical harmonics: 13
    l=0, rc=4.7969 Bohr: 2s-sz confined orbital
    l=1, rc=6.2344 Bohr: 2p-sz confined orbital
    l=0, rc=2.6094 Bohr: 2s-dz split-valence wave
    l=1, rc=3.3594 Bohr: 2p-dz split-valence wave
    l=2, rc=6.2344 Bohr: d-type Gaussian polarization

H-setup:
  name   : Hydrogen
  id     : ea3f9156a1dc40d47a60fdce8f8bd75d
  Z      : 1
  valence: 1
  core   : 0
  charge : 0.0
  file   : /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/H.RPBE.gz
  cutoffs: 0.48(comp), 0.85(filt), 0.53(core), lmax=2
  valence states:
            energy   radius
    1s(1)   -6.572   0.476
    *s      20.639   0.476
    *p       0.000   0.476

LCAO basis set for H:
  Name: dzp
  Basis set was loaded from file /opt/gridware/apps/gcc/gpaw/scalapack/0.9.0+openmpi-1.6.2/share/setups/H.dzp.basis.gz
  Number of radial functions: 3
  Number of spherical harmonics: 5
    l=0, rc=6.4219 Bohr: 1s-sz confined orbital
    l=0, rc=3.6094 Bohr: 1s-dz split-valence wave
    l=1, rc=6.4219 Bohr: p-type Gaussian polarization

Using the RPBE Exchange-Correlation Functional.
Spin-Paired Calculation
Total Charge:      1.000000
Fermi Temperature: 0.050000
Wave functions: Uniform real-space grid
Kinetic energy operator: 6*3+1=19 point O(h^6) finite-difference Laplacian
Eigensolver:       cg
XC and Coulomb potentials evaluated on a 296*288*216 grid
Interpolation: tri-quintic (5. degree polynomial)
Poisson solver: Jacobi solver with 4 multi-grid levels
Stencil: 6*3+1=19 point O(h^6) finite-difference Laplacian
Reference Energy:  -14057566.064888

Total number of cores used: 24
Domain Decomposition: 4 x 3 x 2
MatrixOperator buffer_size: default value or 
                            see value of nblock in input file
Diagonalizer layout: BLACS 3 x 8 grid with 64 x 64 blocksize
Orthonormalizer layout: BLACS 3 x 8 grid with 64 x 64 blocksize

Symmetries present: 1
1 k-point (Gamma)
1 k-point in the Irreducible Part of the Brillouin Zone
Linear Mixing Parameter:           0.05
Pulay Mixing with 5 Old Densities
Damping of Long Wave Oscillations: 100

Convergence Criteria:
Total Energy Change:           0.0005 eV / electron
Integral of Absolute Density Change:    0.0001 electrons
Integral of Absolute Eigenstate Change: 4e-08 eV^2
Number of Atoms: 48
Number of Atomic Orbitals: 395
Number of Bands in Calculation:         272
Bands to Converge:                      Occupied States Only
Number of Valence Electrons:            435
                     log10-error:    Total        Iterations:
           Time      WFS    Density  Energy       Fermi  Poisson
iter:   1  11:54:03  +3.2             793.493507  3      219    
iter:   2  11:59:18  +3.2             694.983740  16            
iter:   3  12:04:34  +3.2             608.411794  12            
iter:   4  12:10:27  +3.3   -0.7      593.116215  28     167    
iter:   5  12:16:13  +3.5   -0.8     -620.885833  7      189    
iter:   6  12:21:45  +4.1   -0.9     -4152.744141  31     200    
iter:   7  12:27:19  +4.0   -1.0     -5087.702212  106    170    
iter:   8  12:32:59  +3.9   -0.7     -5013.659343  82     172    
iter:   9  12:38:35  +3.8   -0.5     -5280.469143  150    136    
iter:  10  12:44:20  +3.6   -0.4     -4046.945751  35     173    
iter:  11  12:50:03  +3.6   -0.3     -5416.635511  57     176    
iter:  12  12:55:48  +3.6   -0.3     -6800.244708  68     177    
iter:  13  13:01:39  +3.4   -0.2     -3197.854429  133    195    
iter:  14  13:07:31  +3.3   -0.2      899.839398  204    203    
iter:  15  13:13:16  +3.3   -0.3     1083.363026  20     197    
iter:  16  13:19:08  +3.5   -0.4     -2328.848545  104    214    
iter:  17  13:24:48  +3.4   -0.3     -417.784506  73     197    
iter:  18  13:30:23  +3.4   -0.3      442.837208  70     164    
iter:  19  13:36:05  +3.1   -0.3      743.492471  65     198    
iter:  20  13:41:50  +3.6   -0.4     -3461.507162  10     214    
iter:  21  13:47:31  +4.4   -0.3     -22064.396389  316    222    
iter:  22  13:53:19  +4.1   -0.1     -10600.579725  226    239    
iter:  23  13:59:01  +3.9   -0.1     -9548.622897  21     196    
iter:  24  14:04:43  +3.9   -0.0     -15930.953088  240    192    
iter:  25  14:10:30  +4.2   +0.0     -35156.510660  4      215    
iter:  26  14:16:09  +4.2   +0.1     -42123.004503  203    186    
iter:  27  14:21:56  +4.5   +0.1     -73815.314101  573    207    
iter:  28  14:27:41  +3.5   +0.2     -6276.066347  157    227    
iter:  29  14:33:28  +4.0   +0.1     1300.429570  415    213    
iter:  30  14:39:09  +3.3   -0.1     1122.221721  52     187    
iter:  31  14:44:51  +3.3   -0.2     -1237.841629  204    189    
iter:  32  14:50:35  +3.4   -0.2      997.101068  324    208    
iter:  33  14:56:05  +4.2   -0.3     -10616.096694  138    223    
iter:  34  15:01:48  +3.7   -0.2     -4946.304627  6      206    
iter:  35  15:07:33  +3.8   -0.1     -11200.304196  180    206    
iter:  36  15:13:16  +3.5   -0.1     -6984.893920  116    202    
iter:  37  15:18:53  +3.5   -0.1     -8118.830881  21     172    
iter:  38  15:24:43  +3.8   -0.1     -21782.429185  377    221    
iter:  39  15:30:27  +3.9   -0.0     -20898.964990  156    197    
iter:  40  15:36:08  +4.0   -0.0     -25342.643988  10     198    
iter:  41  15:41:55  +3.7   -0.0     -17203.969562  178    210    
iter:  42  15:47:40  +3.6   +0.0     -23554.575866  257    202    
iter:  43  15:53:28  +3.5   +0.0     -14057.228383  197    214    
iter:  44  15:59:15  +3.4   +0.0     -6682.048160  244    208    
iter:  45  16:04:58  +3.4   +0.0     -5085.541604  12     195    
iter:  46  16:10:28  +3.4   -0.0     -4407.027801  13     138    
iter:  47  16:16:10  +3.5   -0.0     -12828.036448  201    227    
iter:  48  16:22:00  +3.5   -0.0     -4067.412732  209    222    
iter:  49  16:27:37  +3.2   -0.0     -2218.953433  11     169    
iter:  50  16:33:21  +3.4   -0.1     -3780.705683  4      197    
iter:  51  16:39:08  +3.2   -0.1     -1578.123241  28     215    
iter:  52  16:44:38  +3.7   -0.2     -7800.740717  155    216    
iter:  53  16:50:16  +3.6   -0.1     -4867.753494  11     193    
iter:  54  16:56:02  +3.4   -0.2     -2860.750447  55     206    
iter:  55  17:01:49  +3.4   -0.2     -792.067347  107    210    
iter:  56  17:07:33  +3.3   -0.2     -2004.973347  73     196    
iter:  57  17:13:13  +3.2   -0.2     -1673.304130  6      185    
iter:  58  17:18:45  +3.1   -0.2     -1767.301787  37     144    
iter:  59  17:24:23  +3.1   -0.2     -1293.913967  24     171    
iter:  60  17:29:52  +3.1   -0.2     -1309.144771  13     134    
iter:  61  17:35:28  +3.1   -0.2     -1846.287240  12     165    
iter:  62  17:41:10  +3.0   -0.2     -614.114912  8      188    
iter:  63  17:46:49  +3.0   -0.2     -254.867465  23     177    
iter:  64  17:52:30  +3.0   -0.3      -40.452871  5      183    
iter:  65  17:58:09  +3.1   -0.3     -247.741204  3      182    
iter:  66  18:03:44  +3.2   -0.4     -488.043247  45     165    
iter:  67  18:09:22  +3.3   -0.4     -1312.226795  12     176    
iter:  68  18:14:49  +3.3   -0.3     -1600.650373  36     132    
iter:  69  18:20:24  +3.2   -0.3     -1441.778179  5      158    
iter:  70  18:26:01  +3.2   -0.3     -1091.400632  17     171    
iter:  71  18:31:35  +3.1   -0.3     -1259.417291  15     154    
iter:  72  18:37:13  +3.2   -0.3     -1815.671266  5      172    
iter:  73  18:42:47  +3.2   -0.3     -1680.250148  6      152    
iter:  74  18:48:29  +3.1   -0.3     -687.700911  13     187    
iter:  75  18:53:58  +3.1   -0.3     -781.243980  5      134    
iter:  76  18:59:38  +3.2   -0.3     -287.315654  19     177    
iter:  77  19:05:18  +3.2   -0.3       37.526004  40     178    
iter:  78  19:10:57  +3.2   -0.4      -71.141737  58     181    
iter:  79  19:16:35  +3.3   -0.6     -553.159247  27     171    
iter:  80  19:22:00  +3.2   -0.6     -777.714248  12     117    
iter:  81  19:27:35  +3.2   -0.6     -805.189118  11     157    
iter:  82  19:33:06  +3.2   -0.6     -866.221799  8      142    
iter:  83  19:38:33  +3.2   -0.6     -909.555780  6      122    
iter:  84  19:43:50  +3.2   -0.5     -955.767796  6      82     
iter:  85  19:49:20  +3.2   -0.5     -985.672535  6      134    
iter:  86  19:54:54  +3.2   -0.5     -846.863891  6      157    
iter:  87  20:00:14  +3.2   -0.5     -861.710315  3      93     
iter:  88  20:05:30  +3.2   -0.5     -845.798964  4      78     
iter:  89  20:11:00  +3.2   -0.5     -786.940181  3      137    
iter:  90  20:16:37  +3.2   -0.5     -641.695296  6      164    
iter:  91  20:22:16  +3.2   -0.5     -517.858959  7      176    
iter:  92  20:27:55  +3.3   -0.5     -590.770581  4      177    
iter:  93  20:33:37  +3.4   -0.6     -1207.674805  70     188    
iter:  94  20:39:16  +3.5   -0.6     -2307.667111  97     187    
iter:  95  20:44:52  +3.5   -0.8     -1731.579193  10     174    
iter:  96  20:50:23  +3.5   -0.6     -2156.742513  8      143    
iter:  97  20:55:54  +3.4   -0.5     -2188.063889  15     141    
iter:  98  21:01:28  +3.5   -0.5     -2549.605286  7      156    
iter:  99  21:06:49  +3.4   -0.4     -2620.900033  3      100    
iter: 100  21:12:29  +3.4   -0.4     -2003.308202  10     179    
iter: 101  21:18:05  +3.4   -0.4     -2441.255496  8      163    
iter: 102  21:23:34  +3.5   -0.4     -2517.396918  13     134    
iter: 103  21:29:04  +3.5   -0.4     -2627.324143  12     137    
iter: 104  21:34:41  +3.5   -0.4     -2287.544443  6      166    
iter: 105  21:40:17  +3.5   -0.4     -1986.065262  8      166    
iter: 106  21:45:58  +3.4   -0.4     -1279.500269  14     182    
iter: 107  21:51:38  +3.5   -0.4     -829.165989  38     178    
iter: 108  21:57:24  +3.6   -0.5     -1602.385126  11     206    
iter: 109  22:03:06  +3.3   -0.7     -644.663688  46     187    
iter: 110  22:08:41  +3.3   -0.8     -1193.314368  14     161    
iter: 111  22:14:09  +3.3   -0.7     -1570.714071  6      126    
iter: 112  22:19:30  +3.3   -0.6     -1803.716751  3      100    
iter: 113  22:24:57  +3.3   -0.6     -2049.451257  9      125    
iter: 114  22:30:35  +3.3   -0.5     -1737.030260  3      171    
iter: 115  22:36:03  +3.3   -0.5     -1755.809570  4      129    
iter: 116  22:41:27  +3.4   -0.5     -1783.991369  5      114    
iter: 117  22:46:56  +3.4   -0.5     -1764.055297  5      134    
iter: 118  22:52:34  +3.4   -0.5     -1461.833166  14     172    
iter: 119  22:58:15  +3.4   -0.6     -1177.300913  43     182    
iter: 120  23:03:51  +3.4   -0.6     -1171.693811  20     167    


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